Modern AI acceleration faces a fundamental challenge: conventional assumptions about memory requirements, batching effectiveness, and latency-throughput tradeoffs are systemwide generalizations that ignore the heterogeneous computational patterns of individual neural network operators. However, going towards network-level customization and operator-level heterogeneity incur substantial Non-Recurring Engineering (NRE) costs. While chiplet-based approaches have been proposed to amortize NRE costs, reuse opportunities remain limited without carefully identifying which chiplets are truly necessary. This paper introduces Mozart, a chiplet ecosystem and accelerator codesign framework that systematically constructs low cost bespoke application-specific integrated circuits (BASICs). BASICs leverage operator-level disaggregation to explore chiplet and memory heterogeneity, tensor fusion, and tensor parallelism, with place-and-route validation ensuring physical implementability. The framework also enables constraint-aware system-level optimization across deployment contexts ranging from datacenter inference serving to edge computing in autonomous vehicles. The evaluation confirms that with just 8 strategically selected chiplets, Mozart-generated composite BASICs achieve 43.5%, 25.4%, 67.7%, and 78.8% reductions in energy, energy-cost product, energy-delay product (EDP), and energy-delay-cost product compared to traditional homogeneous accelerators. For datacenter LLM serving, Mozart achieves 15-19% energy reduction and 35-39% energy-cost improvement. In speculative decoding, Mozart delivers throughput improvements of 24.6-58.6% while reducing energy consumption by 38.6-45.6%. For autonomous vehicle perception, Mozart reduces energy-cost by 25.54% and energy by 10.53% under real-time constraints.

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