As NLP models become more complex, understanding their decisions becomes more crucial. Counterfactuals (CFs), where minimal changes to inputs flip a model's prediction, offer a way to explain these models. While Large Language Models (LLMs) have shown remarkable performance in NLP tasks, their efficacy in generating high-quality CFs remains uncertain. This work fills this gap by investigating how well LLMs generate CFs for two NLU tasks. We conduct a comprehensive comparison of several common LLMs, and evaluate their CFs, assessing both intrinsic metrics, and the impact of these CFs on data augmentation. Moreover, we analyze differences between human and LLM-generated CFs, providing insights for future research directions. Our results show that LLMs generate fluent CFs, but struggle to keep the induced changes minimal. Generating CFs for Sentiment Analysis (SA) is less challenging than NLI where LLMs show weaknesses in generating CFs that flip the original label. This also reflects on the data augmentation performance, where we observe a large gap between augmenting with human and LLMs CFs. Furthermore, we evaluate LLMs' ability to assess CFs in a mislabelled data setting, and show that they have a strong bias towards agreeing with the provided labels. GPT4 is more robust against this bias and its scores correlate well with automatic metrics. Our findings reveal several limitations and point to potential future work directions.

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